I would be interested in knowing what books/resources you have found and are reading on the topics of Agile and SCRUM. Also, which did you find to be most informative, intuitive, and overall helpful.
I think documenting invalid scenarios is important. If you don't know how the system should react to invalide scenarios then something is going to break.
I haven't worked a lot with Agile methodologies myself. My knowledge of them is mostly academic.